Articles | Volume 5, issue 1
https://doi.org/10.5194/se-5-409-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/se-5-409-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
BrO/SO2 molar ratios from scanning DOAS measurements in the NOVAC network
P. Lübcke
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Max Planck Institute for Chemistry, Mainz, Germany
N. Bobrowski
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
S. Arellano
Department of Earth and Space Sciences, Chalmers University of Technology, Gothenburg, Sweden
Department of Earth and Space Sciences, Chalmers University of Technology, Gothenburg, Sweden
G. Garzón
FISQUIM Research Group, Laboratory Division, Colombian Geological Survey, Cali, Colombia
L. Vogel
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
now at: Earth Observation Science Group, Space Research Centre, Department of Physics and Astronomy, University of Leicester, Leicester, UK
U. Platt
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
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Simon Warnach, Holger Sihler, Christian Borger, Nicole Bobrowski, Steffen Beirle, Ulrich Platt, and Thomas Wagner
Atmos. Meas. Tech., 16, 5537–5573, https://doi.org/10.5194/amt-16-5537-2023, https://doi.org/10.5194/amt-16-5537-2023, 2023
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Thomas Wagner, Simon Warnach, Steffen Beirle, Nicole Bobrowski, Adrian Jost, Janis Puķīte, and Nicolas Theys
Atmos. Meas. Tech., 16, 1609–1662, https://doi.org/10.5194/amt-16-1609-2023, https://doi.org/10.5194/amt-16-1609-2023, 2023
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Atmos. Meas. Tech., 16, 1343–1356, https://doi.org/10.5194/amt-16-1343-2023, https://doi.org/10.5194/amt-16-1343-2023, 2023
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Optical resonators enhance the light path in compact instruments, thereby improving their sensitivity. Determining the established path length in the instrument is a prerequisite for the accurate determination of trace gas concentrations but can be a significant complication in the use of such resonators. Here we show two calibration techniques which are relatively simple and free of consumables but still provide accurate calibrations. This facilitates the use of optical resonators.
Udo Frieß, Karin Kreher, Richard Querel, Holger Schmithüsen, Dan Smale, Rolf Weller, and Ulrich Platt
Atmos. Chem. Phys., 23, 3207–3232, https://doi.org/10.5194/acp-23-3207-2023, https://doi.org/10.5194/acp-23-3207-2023, 2023
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Reactive bromine compounds, emitted by the sea ice during polar spring, play an important role in the atmospheric chemistry of the coastal regions of Antarctica. We investigate the sources and impacts of reactive bromine in detail using many years of measurements at two Antarctic sites located at opposite sides of the Antarctic continent. Using a multitude of meteorological observations, we were able to identify the main triggers and source regions for reactive bromine in Antarctica.
Maximilian Herrmann, Moritz Schöne, Christian Borger, Simon Warnach, Thomas Wagner, Ulrich Platt, and Eva Gutheil
Atmos. Chem. Phys., 22, 13495–13526, https://doi.org/10.5194/acp-22-13495-2022, https://doi.org/10.5194/acp-22-13495-2022, 2022
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Ozone depletion events (ODEs) are a common occurrence in the boundary layer during Arctic spring. Ozone is depleted by bromine species in an autocatalytic reaction cycle. Previous modeling studies assumed an infinite bromine source at the ground. An alternative emission scheme is presented in which a finite amount of bromide in the snow is tracked over time. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) is used to study ODEs in the Arctic from February to May 2019.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Jan-Lukas Tirpitz, Udo Frieß, Robert Spurr, and Ulrich Platt
Atmos. Meas. Tech., 15, 2077–2098, https://doi.org/10.5194/amt-15-2077-2022, https://doi.org/10.5194/amt-15-2077-2022, 2022
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MAX-DOAS is a widely used measurement technique for the remote detection of atmospheric aerosol and trace gases. It relies on the analysis of ultra-violet and visible radiation spectra of skylight. To date, information contained in the skylight's polarisation state has not been utilised. On the basis of synthetic data, we carried out sensitivity analyses to assess the potential of polarimetry for MAX-DOAS applications.
Leon Kuhn, Jonas Kuhn, Thomas Wagner, and Ulrich Platt
Atmos. Meas. Tech., 15, 1395–1414, https://doi.org/10.5194/amt-15-1395-2022, https://doi.org/10.5194/amt-15-1395-2022, 2022
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Jonas Kuhn, Nicole Bobrowski, Thomas Wagner, and Ulrich Platt
Atmos. Meas. Tech., 14, 7873–7892, https://doi.org/10.5194/amt-14-7873-2021, https://doi.org/10.5194/amt-14-7873-2021, 2021
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Ulrich Platt, Thomas Wagner, Jonas Kuhn, and Thomas Leisner
Atmos. Meas. Tech., 14, 6867–6883, https://doi.org/10.5194/amt-14-6867-2021, https://doi.org/10.5194/amt-14-6867-2021, 2021
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Absorption spectroscopy of scattered sunlight is extremely useful for the analysis of atmospheric trace gas distributions. A central parameter for the achievable sensitivity of spectroscopic instruments is the light throughput, which can be enhanced in a number of ways. We present new ideas and considerations of how instruments could be optimized. Particular emphasis is on arrays of massively parallel instruments. Such arrays can reduce the size and weight of instruments by orders of magnitude.
Alexandra Gutmann, Nicole Bobrowski, Marcello Liotta, and Thorsten Hoffmann
Atmos. Meas. Tech., 14, 6395–6406, https://doi.org/10.5194/amt-14-6395-2021, https://doi.org/10.5194/amt-14-6395-2021, 2021
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Motivated by a special interest in bromine chemistry in volcanic plumes, the study presented here describes a new method for the quantitative collection of gaseous hydrogen bromide in gas diffusion denuders. The hydrogen bromide reacted during sampling with appropriate epoxides applied to the denuder walls. The denuder sampling assembly was successfully deployed in the volcanic plume of Masaya volcano, Nicaragua.
Florian Dinger, Timo Kleinbek, Steffen Dörner, Nicole Bobrowski, Ulrich Platt, Thomas Wagner, Martha Ibarra, and Eveling Espinoza
Atmos. Chem. Phys., 21, 9367–9404, https://doi.org/10.5194/acp-21-9367-2021, https://doi.org/10.5194/acp-21-9367-2021, 2021
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Monitoring magnitude or chemical composition of volcanic gas emissions can help to forecast volcanic eruptions and provides empirical data on the impact of volcanoes on the chemistry in the local and global atmosphere. This study reports and discusses continuous time series of the sulfur and bromine emission fluxes of Masaya from 2014 to 2020. We observed an annual cyclicity in the BrO / SO2 molar ratio, possibly caused by the annual variability in the atmospheric humidity.
Bo Galle, Santiago Arellano, Nicole Bobrowski, Vladimir Conde, Tobias P. Fischer, Gustav Gerdes, Alexandra Gutmann, Thorsten Hoffmann, Ima Itikarai, Tomas Krejci, Emma J. Liu, Kila Mulina, Scott Nowicki, Tom Richardson, Julian Rüdiger, Kieran Wood, and Jiazhi Xu
Atmos. Meas. Tech., 14, 4255–4277, https://doi.org/10.5194/amt-14-4255-2021, https://doi.org/10.5194/amt-14-4255-2021, 2021
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Measurements of volcanic gases are important for geophysical research, risk assessment and environmental impact studies. Some gases, like SO2 and BrO, may be studied from the ground at a safe distance using remote sensing techniques. Many other gases require in situ access to the gas plume. Here, a drone may be an attractive alternative. This paper describes a drone specially adapted for volcanic gas studies and demonstrates its use in a field campaign at Manam volcano in Papua New Guinea.
Maximilian Herrmann, Holger Sihler, Udo Frieß, Thomas Wagner, Ulrich Platt, and Eva Gutheil
Atmos. Chem. Phys., 21, 7611–7638, https://doi.org/10.5194/acp-21-7611-2021, https://doi.org/10.5194/acp-21-7611-2021, 2021
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Time-dependent 3D numerical simulations of tropospheric bromine release and ozone depletion events (ODEs) in the Arctic polar spring of 2009 are compared to observations. Simulation results agree well with the observations at both Utqiaġvik, Alaska, and at Summit, Greenland. In a parameter study, different settings for the bromine release mechanism are evaluated. An enhancement of the bromine release mechanism improves the agreement regarding the occurrence of ODEs with the observations.
Santiago Arellano, Bo Galle, Fredy Apaza, Geoffroy Avard, Charlotte Barrington, Nicole Bobrowski, Claudia Bucarey, Viviana Burbano, Mike Burton, Zoraida Chacón, Gustavo Chigna, Christian Joseph Clarito, Vladimir Conde, Fidel Costa, Maarten De Moor, Hugo Delgado-Granados, Andrea Di Muro, Deborah Fernandez, Gustavo Garzón, Hendra Gunawan, Nia Haerani, Thor H. Hansteen, Silvana Hidalgo, Salvatore Inguaggiato, Mattias Johansson, Christoph Kern, Manne Kihlman, Philippe Kowalski, Pablo Masias, Francisco Montalvo, Joakim Möller, Ulrich Platt, Claudia Rivera, Armando Saballos, Giuseppe Salerno, Benoit Taisne, Freddy Vásconez, Gabriela Velásquez, Fabio Vita, and Mathieu Yalire
Earth Syst. Sci. Data, 13, 1167–1188, https://doi.org/10.5194/essd-13-1167-2021, https://doi.org/10.5194/essd-13-1167-2021, 2021
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This study presents a dataset of volcanic sulfur dioxide (SO2) emissions from 2005–2017. Measurements were obtained by Network for Observation of Volcanic and Atmospheric Change (NOVAC) scanning differential optical absorption spectrometer (ScanDOAS) instruments at 32 volcanoes and processed using a standardized procedure. We show statistics of volcanic gas emissions under a variety of conditions and compare them with averages derived from measurements from space and historical inventories.
Julian Rüdiger, Alexandra Gutmann, Nicole Bobrowski, Marcello Liotta, J. Maarten de Moor, Rolf Sander, Florian Dinger, Jan-Lukas Tirpitz, Martha Ibarra, Armando Saballos, María Martínez, Elvis Mendoza, Arnoldo Ferrufino, John Stix, Juan Valdés, Jonathan M. Castro, and Thorsten Hoffmann
Atmos. Chem. Phys., 21, 3371–3393, https://doi.org/10.5194/acp-21-3371-2021, https://doi.org/10.5194/acp-21-3371-2021, 2021
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We present an innovative approach to study halogen chemistry in the plume of Masaya volcano in Nicaragua. An unique data set was collected using multiple techniques, including drones. These data enabled us to determine the fraction of activation of the respective halogens at various plume ages, where in-mixing of ambient air causes chemical reactions. An atmospheric chemistry box model was employed to further examine the field results and help our understanding of volcanic plume chemistry.
Christopher Fuchs, Jonas Kuhn, Nicole Bobrowski, and Ulrich Platt
Atmos. Meas. Tech., 14, 295–307, https://doi.org/10.5194/amt-14-295-2021, https://doi.org/10.5194/amt-14-295-2021, 2021
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We present first measurements of volcanic SO2 emissions with a novel imaging technique for atmospheric trace gases in the UV and visible spectral range. Periodic spectral Fabry–Pérot interferometer transmission features are matched to differential absorption cross sections of the investigated trace gas, yielding high selectivity and sensitivity. The technique can be extended to measure many other trace gases with high spatio-temporal resolution.
Jan-Lukas Tirpitz, Udo Frieß, François Hendrick, Carlos Alberti, Marc Allaart, Arnoud Apituley, Alkis Bais, Steffen Beirle, Stijn Berkhout, Kristof Bognar, Tim Bösch, Ilya Bruchkouski, Alexander Cede, Ka Lok Chan, Mirjam den Hoed, Sebastian Donner, Theano Drosoglou, Caroline Fayt, Martina M. Friedrich, Arnoud Frumau, Lou Gast, Clio Gielen, Laura Gomez-Martín, Nan Hao, Arjan Hensen, Bas Henzing, Christian Hermans, Junli Jin, Karin Kreher, Jonas Kuhn, Johannes Lampel, Ang Li, Cheng Liu, Haoran Liu, Jianzhong Ma, Alexis Merlaud, Enno Peters, Gaia Pinardi, Ankie Piters, Ulrich Platt, Olga Puentedura, Andreas Richter, Stefan Schmitt, Elena Spinei, Deborah Stein Zweers, Kimberly Strong, Daan Swart, Frederik Tack, Martin Tiefengraber, René van der Hoff, Michel van Roozendael, Tim Vlemmix, Jan Vonk, Thomas Wagner, Yang Wang, Zhuoru Wang, Mark Wenig, Matthias Wiegner, Folkard Wittrock, Pinhua Xie, Chengzhi Xing, Jin Xu, Margarita Yela, Chengxin Zhang, and Xiaoyi Zhao
Atmos. Meas. Tech., 14, 1–35, https://doi.org/10.5194/amt-14-1-2021, https://doi.org/10.5194/amt-14-1-2021, 2021
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Multi-axis differential optical absorption spectroscopy (MAX-DOAS) is a ground-based remote sensing measurement technique that derives atmospheric aerosol and trace gas vertical profiles from skylight spectra. In this study, consistency and reliability of MAX-DOAS profiles are assessed by applying nine different evaluation algorithms to spectral data recorded during an intercomparison campaign in the Netherlands and by comparing the results to colocated supporting observations.
Karin Kreher, Michel Van Roozendael, Francois Hendrick, Arnoud Apituley, Ermioni Dimitropoulou, Udo Frieß, Andreas Richter, Thomas Wagner, Johannes Lampel, Nader Abuhassan, Li Ang, Monica Anguas, Alkis Bais, Nuria Benavent, Tim Bösch, Kristof Bognar, Alexander Borovski, Ilya Bruchkouski, Alexander Cede, Ka Lok Chan, Sebastian Donner, Theano Drosoglou, Caroline Fayt, Henning Finkenzeller, David Garcia-Nieto, Clio Gielen, Laura Gómez-Martín, Nan Hao, Bas Henzing, Jay R. Herman, Christian Hermans, Syedul Hoque, Hitoshi Irie, Junli Jin, Paul Johnston, Junaid Khayyam Butt, Fahim Khokhar, Theodore K. Koenig, Jonas Kuhn, Vinod Kumar, Cheng Liu, Jianzhong Ma, Alexis Merlaud, Abhishek K. Mishra, Moritz Müller, Monica Navarro-Comas, Mareike Ostendorf, Andrea Pazmino, Enno Peters, Gaia Pinardi, Manuel Pinharanda, Ankie Piters, Ulrich Platt, Oleg Postylyakov, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Alfonso Saiz-Lopez, Anja Schönhardt, Stefan F. Schreier, André Seyler, Vinayak Sinha, Elena Spinei, Kimberly Strong, Frederik Tack, Xin Tian, Martin Tiefengraber, Jan-Lukas Tirpitz, Jeroen van Gent, Rainer Volkamer, Mihalis Vrekoussis, Shanshan Wang, Zhuoru Wang, Mark Wenig, Folkard Wittrock, Pinhua H. Xie, Jin Xu, Margarita Yela, Chengxin Zhang, and Xiaoyi Zhao
Atmos. Meas. Tech., 13, 2169–2208, https://doi.org/10.5194/amt-13-2169-2020, https://doi.org/10.5194/amt-13-2169-2020, 2020
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In September 2016, 36 spectrometers from 24 institutes measured a number of key atmospheric pollutants during an instrument intercomparison campaign (CINDI-2) at Cabauw, the Netherlands. Here we report on the outcome of this intercomparison exercise. The three major goals were to characterise the differences between the participating instruments, to define a robust methodology for performance assessment, and to contribute to the harmonisation of the measurement settings and retrieval methods.
Ulrich Platt and Jonas Kuhn
Atmos. Meas. Tech., 12, 6259–6272, https://doi.org/10.5194/amt-12-6259-2019, https://doi.org/10.5194/amt-12-6259-2019, 2019
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Measurements of atmospheric trace gases by absorption spectroscopy are frequently supported by recording the amount of trace gas in absorption cells. These are typically small glass (or quartz) cylinders containing the gas to be studied. Here we show in the example of NO2-absorption cells that the effective amount of gas seen by the instrument can deviate greatly from expected values (by orders of magnitude in severe cases). Some suggestions for improving the situation are discussed.
Maximilian Herrmann, Le Cao, Holger Sihler, Ulrich Platt, and Eva Gutheil
Atmos. Chem. Phys., 19, 10161–10190, https://doi.org/10.5194/acp-19-10161-2019, https://doi.org/10.5194/acp-19-10161-2019, 2019
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The oscillations of tropospheric ODEs in the Arctic spring is studied numerically. After the termination of an ODE, the reactive bromine is deposited onto aerosols/the snow surface, and the ozone may regenerate. The replenished ozone is available for the next autocatalytic bromine release, leading to the oscillation of an ODE. Its dependence on the NOx mixing ratio, the inversion layer strength, the ambient temperature, the aerosol density, and the solar radiation is investigated.
Jan-Marcus Nasse, Philipp G. Eger, Denis Pöhler, Stefan Schmitt, Udo Frieß, and Ulrich Platt
Atmos. Meas. Tech., 12, 4149–4169, https://doi.org/10.5194/amt-12-4149-2019, https://doi.org/10.5194/amt-12-4149-2019, 2019
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We present several changes to the setup of long-path differential optical absorption spectroscopy (LP-DOAS) instruments, including the application of a laser-driven light source, a modified coupling of the measurement signal between components, improved stray-light suppression, and better signal homogenization measures. These changes reduce detection limits of typical trace-gas species by a factor of 3–4 compared to previous setups and enable automated long-term observations in Antarctica.
Martin Horbanski, Denis Pöhler, Johannes Lampel, and Ulrich Platt
Atmos. Meas. Tech., 12, 3365–3381, https://doi.org/10.5194/amt-12-3365-2019, https://doi.org/10.5194/amt-12-3365-2019, 2019
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ICAD allows a precise in situ measurement of gases like NO2 in a relatively simple and compact setup. The main advantage in comparison to most other optical methods is that it does not require a stable total light intensity. This allows a simpler and mobile instrument setup and additionally it features no observed cross-interferences. We validated the high quality for an ICAD NO2 instrument in different inter-comparisons with a detection limit of 0.02 ppbv.
Florian Dinger, Stefan Bredemeyer, Santiago Arellano, Nicole Bobrowski, Ulrich Platt, and Thomas Wagner
Solid Earth, 10, 725–740, https://doi.org/10.5194/se-10-725-2019, https://doi.org/10.5194/se-10-725-2019, 2019
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Evidence for tidal impacts on volcanism have been gathered by numerous empirical studies. This paper elucidates whether a causal link from the tidal forces to a variation in the volcanic degassing can be traced analytically. We model the response of a simplified magmatic system to the local tidal gravity variations, find that the tide-induced dynamics may significantly alter the bubble coalescence rate, and discuss the consequences for volcanic degassing behaviour.
Jonas Kuhn, Ulrich Platt, Nicole Bobrowski, and Thomas Wagner
Atmos. Meas. Tech., 12, 735–747, https://doi.org/10.5194/amt-12-735-2019, https://doi.org/10.5194/amt-12-735-2019, 2019
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We study a novel remote-sensing technique for atmospheric trace gases absorbing in the UV and visible spectral range. Using Fabry–Perot interferometers with a spectral transmission matched to the trace gas's spectral absorption allows for imaging trace gases with high sensitivity and selectivity. The thereby achieved high spatio-temporal resolution enables the study of small-scale and dynamic processes in the atmosphere. We present sample calculations and a proof-of-concept study.
Jorge Saturno, Florian Ditas, Marloes Penning de Vries, Bruna A. Holanda, Mira L. Pöhlker, Samara Carbone, David Walter, Nicole Bobrowski, Joel Brito, Xuguang Chi, Alexandra Gutmann, Isabella Hrabe de Angelis, Luiz A. T. Machado, Daniel Moran-Zuloaga, Julian Rüdiger, Johannes Schneider, Christiane Schulz, Qiaoqiao Wang, Manfred Wendisch, Paulo Artaxo, Thomas Wagner, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10391–10405, https://doi.org/10.5194/acp-18-10391-2018, https://doi.org/10.5194/acp-18-10391-2018, 2018
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This study uses satellite observations to track volcanic emissions in eastern Congo and their subsequent transport across the Atlantic Ocean into the Amazon Basin. Aircraft and ground-based observations are used to characterize the influence of volcanogenic aerosol on the chemical and microphysical properties of Amazonian aerosols. Further, this work is an illustrative example of the conditions and dynamics driving the transatlantic transport of African emissions to South America.
Stephen Broccardo, Klaus-Peter Heue, David Walter, Christian Meyer, Alexander Kokhanovsky, Ronald van der A, Stuart Piketh, Kristy Langerman, and Ulrich Platt
Atmos. Meas. Tech., 11, 2797–2819, https://doi.org/10.5194/amt-11-2797-2018, https://doi.org/10.5194/amt-11-2797-2018, 2018
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Measurements of nitrogen dioxide, known to originate from industrial and automotive combustion sources, have been made from space for two decades. Successive generations of instrument bring improvements in ground-pixel resolution; however features in the atmosphere are known to be smaller than what the satellites can resolve. Measurements of urban and industrial areas using a high-resolution airborne instrument allow the impact of the satellite's relatively low resolution to be evaluated.
Julian Rüdiger, Jan-Lukas Tirpitz, J. Maarten de Moor, Nicole Bobrowski, Alexandra Gutmann, Marco Liuzzo, Martha Ibarra, and Thorsten Hoffmann
Atmos. Meas. Tech., 11, 2441–2457, https://doi.org/10.5194/amt-11-2441-2018, https://doi.org/10.5194/amt-11-2441-2018, 2018
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Volcanic gas emission studies are important for monitoring active volcanoes, obtaining insights into subsurface processes and opening up an interesting domain for atmospheric chemistry investigations. Using an unmanned aerial vehicle, commonly called a drone, we were able to study various volcanic gases at sites which are typically too dangerous to access otherwise. The use of drones for volcano monitoring and gas measurements in harsh environments was successfully assessed.
David W. T. Griffith, Denis Pöhler, Stefan Schmitt, Samuel Hammer, Sanam N. Vardag, and Ulrich Platt
Atmos. Meas. Tech., 11, 1549–1563, https://doi.org/10.5194/amt-11-1549-2018, https://doi.org/10.5194/amt-11-1549-2018, 2018
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Measurements of atmospheric trace gases over an open path complement in situ measurements by spatial averaging. This paper describes the first open-path measurements of CO2, CH4 and other trace gases by near-infrared Fourier transform spectroscopy. The measurements were made in Heidelberg, Germany, for 4 months in 2014 over a 1.5 km path and compared to in situ measurements made at one end of the path. The experiment setup and methods (and the comparisons of open path to in situ) are described.
Florian Dinger, Nicole Bobrowski, Simon Warnach, Stefan Bredemeyer, Silvana Hidalgo, Santiago Arellano, Bo Galle, Ulrich Platt, and Thomas Wagner
Solid Earth, 9, 247–266, https://doi.org/10.5194/se-9-247-2018, https://doi.org/10.5194/se-9-247-2018, 2018
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We monitored the bromine monoxide-to-sulfur dioxide molar ratio in the effusive gas plume of Cotopaxi volcano in order to gain insight into the geological processes which control the pressure regime of the volcanic system. We observed a conspicuous periodic pattern with a periodicity of about 2 weeks, which significantly correlates with the Earth tidal forcing. Our results support a possible Earth tidal impact on volcanic activity, in particular for the Cotopaxi eruption 2015.
Christoph Kleinschmitt, Olivier Boucher, and Ulrich Platt
Atmos. Chem. Phys., 18, 2769–2786, https://doi.org/10.5194/acp-18-2769-2018, https://doi.org/10.5194/acp-18-2769-2018, 2018
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We use a state-of-the-art stratospheric aerosol model to study geoengineering through stratospheric sulfur injections. We find that the efficiency may decrease more drastically for larger injections than previously estimated and that injections at higher altitude are not more effective. This study may provide additional evidence that this proposed geoengineering technique is still more complicated, probably less effective, and may implicate stronger side effects than initially thought.
Johannes Lampel, Johannes Zielcke, Stefan Schmitt, Denis Pöhler, Udo Frieß, Ulrich Platt, and Thomas Wagner
Atmos. Chem. Phys., 18, 1671–1683, https://doi.org/10.5194/acp-18-1671-2018, https://doi.org/10.5194/acp-18-1671-2018, 2018
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Previous publications on the absorptions of the oxygen dimer O2–O2 (or short: O4) list absorption peaks at 328 nm and 419 nm, for which no spectrally resolved literature cross sections are available. As these absorptions potentially influence the spectral retrieval of various other trace gases, their shape and magnitude need to be quantified. We approximate the absorption peaks at 328 nm and 419 nm by their respective neighboring absorption peaks to estimate their magnitude and peak wavelength.
Johannes Lampel, Yang Wang, Andreas Hilboll, Steffen Beirle, Holger Sihler, Janis Puķīte, Ulrich Platt, and Thomas Wagner
Atmos. Meas. Tech., 10, 4819–4831, https://doi.org/10.5194/amt-10-4819-2017, https://doi.org/10.5194/amt-10-4819-2017, 2017
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Experience of differential atmospheric absorption spectroscopy (DOAS) shows that a spectral shift between measurement and reference spectrum is frequently required in order to achieve optimal fit results. The shift is often attributed to temporal instabilities of the instrument but implicitly solved the problem of the tilt effect discussed in this paper. The tilt effect results from the finite resolution of the measurements and amounts to 2 pm for the example data set.
Christoph Kleinschmitt, Olivier Boucher, Slimane Bekki, François Lott, and Ulrich Platt
Geosci. Model Dev., 10, 3359–3378, https://doi.org/10.5194/gmd-10-3359-2017, https://doi.org/10.5194/gmd-10-3359-2017, 2017
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Stratospheric aerosols play an important role in the climate system by affecting the Earth's radiative budget. In this article we present the newly developed LMDZ-S3A model and assess its performance against observations in periods of low and high aerosol loading. The model may serve as a tool to study the climate impacts of volcanic eruptions, as well as the deliberate injection of aerosols into the stratosphere, which has been proposed as a method of geoengineering to abate global warming.
William R. Simpson, Peter K. Peterson, Udo Frieß, Holger Sihler, Johannes Lampel, Ulrich Platt, Chris Moore, Kerri Pratt, Paul Shepson, John Halfacre, and Son V. Nghiem
Atmos. Chem. Phys., 17, 9291–9309, https://doi.org/10.5194/acp-17-9291-2017, https://doi.org/10.5194/acp-17-9291-2017, 2017
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We investigated Arctic atmospheric bromine chemistry during March–April 2012 to improve understanding of the role of sea ice and cracks in sea ice (leads) in this phenomenon. We find that leads vertically redistribute reactive bromine but that open/re-freezing leads are not major direct reactive halogen sources. Surface ozone depletion affects the vertical distribution and amount of reactive halogens, and aerosol particles are necessary but not sufficient to maintain reactive bromine aloft.
Peter K. Peterson, Denis Pöhler, Holger Sihler, Johannes Zielcke, Stephan General, Udo Frieß, Ulrich Platt, William R. Simpson, Son V. Nghiem, Paul B. Shepson, Brian H. Stirm, Suresh Dhaniyala, Thomas Wagner, Dana R. Caulton, Jose D. Fuentes, and Kerri A. Pratt
Atmos. Chem. Phys., 17, 7567–7579, https://doi.org/10.5194/acp-17-7567-2017, https://doi.org/10.5194/acp-17-7567-2017, 2017
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High-spatial-resolution aircraft measurements in the Arctic showed the sustained transport of reactive bromine in a lofted layer via heterogeneous reactions on aerosol particles. This process provides an explanation for free tropospheric reactive bromine and the significant spatial extent of satellite-observed bromine monoxide. The knowledge gained herein improves our understanding of the fate and transport of atmospheric pollutants in the Arctic.
Pierre Tulet, Andréa Di Muro, Aurélie Colomb, Cyrielle Denjean, Valentin Duflot, Santiago Arellano, Brice Foucart, Jérome Brioude, Karine Sellegri, Aline Peltier, Alessandro Aiuppa, Christelle Barthe, Chatrapatty Bhugwant, Soline Bielli, Patrice Boissier, Guillaume Boudoire, Thierry Bourrianne, Christophe Brunet, Fréderic Burnet, Jean-Pierre Cammas, Franck Gabarrot, Bo Galle, Gaetano Giudice, Christian Guadagno, Fréderic Jeamblu, Philippe Kowalski, Jimmy Leclair de Bellevue, Nicolas Marquestaut, Dominique Mékies, Jean-Marc Metzger, Joris Pianezze, Thierry Portafaix, Jean Sciare, Arnaud Tournigand, and Nicolas Villeneuve
Atmos. Chem. Phys., 17, 5355–5378, https://doi.org/10.5194/acp-17-5355-2017, https://doi.org/10.5194/acp-17-5355-2017, 2017
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The STRAP campaign was conducted in 2015 to investigate the volcanic plumes of Piton de La Fournaise (La Réunion, France). For the first time, measurements were conducted at the local (near the vent) and regional scales around the island. The STRAP 2015 campaign gave a unique set of multi-disciplinary data that can now be used by modellers to improve the numerical parameterisations of the physical and chemical evolution of the volcanic plumes.
Angelika Klein, Peter Lübcke, Nicole Bobrowski, Jonas Kuhn, and Ulrich Platt
Atmos. Meas. Tech., 10, 979–987, https://doi.org/10.5194/amt-10-979-2017, https://doi.org/10.5194/amt-10-979-2017, 2017
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While measuring sulfur dioxide fluxes in volcanic plumes with a UV-sensitive camera, the wind direction can influence the retrieved fluxes. If the volcanic plume is tilted in the field of view of the camera, it can lead to over- or underestimations of the determined fluxes. This paper presents a method to deal with such a circumstance. Additionally, it provides the possibility to determine the wind direction of the plume directly from the image time series themselves.
Nga Lee Ng, Steven S. Brown, Alexander T. Archibald, Elliot Atlas, Ronald C. Cohen, John N. Crowley, Douglas A. Day, Neil M. Donahue, Juliane L. Fry, Hendrik Fuchs, Robert J. Griffin, Marcelo I. Guzman, Hartmut Herrmann, Alma Hodzic, Yoshiteru Iinuma, José L. Jimenez, Astrid Kiendler-Scharr, Ben H. Lee, Deborah J. Luecken, Jingqiu Mao, Robert McLaren, Anke Mutzel, Hans D. Osthoff, Bin Ouyang, Benedicte Picquet-Varrault, Ulrich Platt, Havala O. T. Pye, Yinon Rudich, Rebecca H. Schwantes, Manabu Shiraiwa, Jochen Stutz, Joel A. Thornton, Andreas Tilgner, Brent J. Williams, and Rahul A. Zaveri
Atmos. Chem. Phys., 17, 2103–2162, https://doi.org/10.5194/acp-17-2103-2017, https://doi.org/10.5194/acp-17-2103-2017, 2017
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Oxidation of biogenic volatile organic compounds by NO3 is an important interaction between anthropogenic
and natural emissions. This review results from a June 2015 workshop and includes the recent literature
on kinetics, mechanisms, organic aerosol yields, and heterogeneous chemistry; advances in analytical
instrumentation; the current state NO3-BVOC chemistry in atmospheric models; and critical needs for
future research in modeling, field observations, and laboratory studies.
Johannes Lampel, Denis Pöhler, Oleg L. Polyansky, Aleksandra A. Kyuberis, Nikolai F. Zobov, Jonathan Tennyson, Lorenzo Lodi, Udo Frieß, Yang Wang, Steffen Beirle, Ulrich Platt, and Thomas Wagner
Atmos. Chem. Phys., 17, 1271–1295, https://doi.org/10.5194/acp-17-1271-2017, https://doi.org/10.5194/acp-17-1271-2017, 2017
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Water vapour is known to absorb radiation from the microwave region to the blue part of the visible spectrum.
Ab initio approaches to model individual absorption lines of the gaseous water molecule predict absorption lines
until its dissociation limit at 243 nm.
We present first evidence of water vapour absorption near 363 nm from field measurements using data
from multi-axis differential optical absorption spectroscopy (MAX-DOAS) and long-path (LP)-DOAS measurements.
André Butz, Anna Solvejg Dinger, Nicole Bobrowski, Julian Kostinek, Lukas Fieber, Constanze Fischerkeller, Giovanni Bruno Giuffrida, Frank Hase, Friedrich Klappenbach, Jonas Kuhn, Peter Lübcke, Lukas Tirpitz, and Qiansi Tu
Atmos. Meas. Tech., 10, 1–14, https://doi.org/10.5194/amt-10-1-2017, https://doi.org/10.5194/amt-10-1-2017, 2017
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Remote sensing of the gaseous composition of non-eruptive, passively degassing volcanic plumes can be a tool for volcano monitoring. Here, we report on a field study that demonstrates the feasibility of remotely measuring the volcanic enhancements of carbon dioxide, hydrogen fluoride, hydrogen chloride, sulfur dioxide, and bromine monoxide in the plume of Mt. Etna using portable spectroscopic instrumentation sampling the plume several kilometers downwind of the source.
Peter Lübcke, Johannes Lampel, Santiago Arellano, Nicole Bobrowski, Florian Dinger, Bo Galle, Gustavo Garzón, Silvana Hidalgo, Zoraida Chacón Ortiz, Leif Vogel, Simon Warnach, and Ulrich Platt
Atmos. Meas. Tech., 9, 5677–5698, https://doi.org/10.5194/amt-9-5677-2016, https://doi.org/10.5194/amt-9-5677-2016, 2016
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We evaluated spectra from a scanning spectrometer network for the monitoring of volcanic gas emissions using a modelled background spectrum. Statistical methods were applied in order to improve the quality of the spectroscopic evaluation. We used this technique to assess the robustness of standard retrievals at two volcanos: Nevado del Ruiz (Colombia) and Tungurahua (Ecuador).
Christoph Hörmann, Holger Sihler, Steffen Beirle, Marloes Penning de Vries, Ulrich Platt, and Thomas Wagner
Atmos. Chem. Phys., 16, 13015–13034, https://doi.org/10.5194/acp-16-13015-2016, https://doi.org/10.5194/acp-16-13015-2016, 2016
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We present 10 years of bromine monoxide (BrO) satellite observations by the Ozone Monitoring Instrument (OMI) over the Rann of Kutch salt marsh. The measurements reveal a typical seasonal cycle of BrO with maximum concentrations during April/May. The results indicate that the Rann of Kutch is probably one of the strongest natural point sources of reactive bromine compounds outside the polar regions and is thought to have a significant impact on local and regional ozone chemistry.
Erna Frins, Reza Shaiganfar, Ulrich Platt, and Thomas Wagner
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-255, https://doi.org/10.5194/amt-2016-255, 2016
Revised manuscript has not been submitted
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Standard methods like in-situ measurements can hardly register NOx (= NO + NO2) emissions from aircrafts during take-off, when engines run at high load and thus an important amount of fuel is consumed and most of the harmful emissions are produced . The goal of this work is to show that it is possible to measure aircraft emissions generated during take-off (and initial part of the climb) by a remote spectroscopic method like automobile – based – Differential Optical Absorption Spectroscopy (DOAS).
Le Cao, Ulrich Platt, Chenggang Wang, Nianwen Cao, and Qing Qin
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-553, https://doi.org/10.5194/acp-2016-553, 2016
Revised manuscript has not been submitted
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A snowpack module which represents the mass transfer between the ambient air and the snowpack is implemented in a box model, aiming to clarify the influences of the snowpack on the ozone depletion events (ODEs) and the associated bromine explosion in the springtime of Arctic. The size of snow grains, volume fraction of the liquid-like layer (LLL), and the rate of the mass exchange between the snow interstitial air and the snow particles are shown to be critical parameters.
N. Sobanski, M. J. Tang, J. Thieser, G. Schuster, D. Pöhler, H. Fischer, W. Song, C. Sauvage, J. Williams, J. Fachinger, F. Berkes, P. Hoor, U. Platt, J. Lelieveld, and J. N. Crowley
Atmos. Chem. Phys., 16, 4867–4883, https://doi.org/10.5194/acp-16-4867-2016, https://doi.org/10.5194/acp-16-4867-2016, 2016
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The nitrate radical (NO3) is an important nocturnal oxidant. By measuring NO3, its precursors (nitrogen dioxide and ozone) and several trace gases with which it reacts, we examined the chemical and meteorological factors influencing the lifetime of NO3 at a semi-rural mountain site. Unexpectedly long lifetimes, approaching 1 h, were observed on several nights and were associated with a low-lying residual layer. We discuss the role of other reactions that convert NO2 to NO3.
J. Lampel, D. Pöhler, J. Tschritter, U. Frieß, and U. Platt
Atmos. Meas. Tech., 8, 4329–4346, https://doi.org/10.5194/amt-8-4329-2015, https://doi.org/10.5194/amt-8-4329-2015, 2015
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In recent updates of the HITRAN water vapour H2O spectroscopic compilation covering the blue spectral region (here 394–-480 nm) significant changes for the absorption bands at 416 and 426 nm were reported. In order to investigate the consistency of the different cross sections calculated from these compilations, H2O vapour column density ratios for different spectral intervals were retrieved from long-path and multi-axis differential optical absorption spectroscopy measurements.
K. D. Custard, C. R. Thompson, K. A. Pratt, P B. Shepson, J. Liao, L. G. Huey, J. J. Orlando, A. J. Weinheimer, E. Apel, S. R. Hall, F. Flocke, L. Mauldin, R. S. Hornbrook, D. Pöhler, S. General, J. Zielcke, W. R. Simpson, U. Platt, A. Fried, P. Weibring, B. C. Sive, K. Ullmann, C. Cantrell, D. J. Knapp, and D. D. Montzka
Atmos. Chem. Phys., 15, 10799–10809, https://doi.org/10.5194/acp-15-10799-2015, https://doi.org/10.5194/acp-15-10799-2015, 2015
J. Lampel, U. Frieß, and U. Platt
Atmos. Meas. Tech., 8, 3767–3787, https://doi.org/10.5194/amt-8-3767-2015, https://doi.org/10.5194/amt-8-3767-2015, 2015
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In remote sensing applications, such as differential optical absorption spectroscopy (DOAS), atmospheric scattering processes need to be considered. Inelastic scattering on air molecules can lead to filling-in of absorption lines. The contribution of rotational Raman scattering is typically corrected for. The magnitude of vibrational Raman scattering (VRS) is known from theory and agrees with our first DOAS observations of this effect. Its impact on trace-gas measurements of NO2 is discussed.
J. Gliß, N. Bobrowski, L. Vogel, D. Pöhler, and U. Platt
Atmos. Chem. Phys., 15, 5659–5681, https://doi.org/10.5194/acp-15-5659-2015, https://doi.org/10.5194/acp-15-5659-2015, 2015
P. K. Peterson, W. R. Simpson, K. A. Pratt, P. B. Shepson, U. Frieß, J. Zielcke, U. Platt, S. J. Walsh, and S. V. Nghiem
Atmos. Chem. Phys., 15, 2119–2137, https://doi.org/10.5194/acp-15-2119-2015, https://doi.org/10.5194/acp-15-2119-2015, 2015
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We developed methods to measure the vertical distribution of bromine monoxide, a gas that oxidizes pollutants, above sea ice based upon MAX-DOAS observations from Barrow, Alaska, and find that atmospheric stability exerts a strong control on BrO's vertical distribution. Specifically, more stable (temperature inversion) situations result in BrO being closer to the ground while more neutral (not inverted) atmospheres allow BrO to ascend further aloft and grow to larger column abundance.
J. Kuhn, N. Bobrowski, P. Lübcke, L. Vogel, and U. Platt
Atmos. Meas. Tech., 7, 3705–3715, https://doi.org/10.5194/amt-7-3705-2014, https://doi.org/10.5194/amt-7-3705-2014, 2014
S. General, D. Pöhler, H. Sihler, N. Bobrowski, U. Frieß, J. Zielcke, M. Horbanski, P. B. Shepson, B. H. Stirm, W. R. Simpson, K. Weber, C. Fischer, and U. Platt
Atmos. Meas. Tech., 7, 3459–3485, https://doi.org/10.5194/amt-7-3459-2014, https://doi.org/10.5194/amt-7-3459-2014, 2014
V. Conde, D. Nilsson, B. Galle, R. Cartagena, and A. Muñoz
Geosci. Instrum. Method. Data Syst., 3, 127–134, https://doi.org/10.5194/gi-3-127-2014, https://doi.org/10.5194/gi-3-127-2014, 2014
K.-P. Heue, H. Riede, D. Walter, C. A. M. Brenninkmeijer, T. Wagner, U. Frieß, U. Platt, A. Zahn, G. Stratmann, and H. Ziereis
Atmos. Chem. Phys., 14, 6621–6642, https://doi.org/10.5194/acp-14-6621-2014, https://doi.org/10.5194/acp-14-6621-2014, 2014
S. Bleicher, J. C. Buxmann, R. Sander, T. P. Riedel, J. A. Thornton, U. Platt, and C. Zetzsch
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-10135-2014, https://doi.org/10.5194/acpd-14-10135-2014, 2014
Revised manuscript has not been submitted
L. Cao, H. Sihler, U. Platt, and E. Gutheil
Atmos. Chem. Phys., 14, 3771–3787, https://doi.org/10.5194/acp-14-3771-2014, https://doi.org/10.5194/acp-14-3771-2014, 2014
C. Liu, S. Beirle, T. Butler, P. Hoor, C. Frankenberg, P. Jöckel, M. Penning de Vries, U. Platt, A. Pozzer, M. G. Lawrence, J. Lelieveld, H. Tost, and T. Wagner
Atmos. Chem. Phys., 14, 1717–1732, https://doi.org/10.5194/acp-14-1717-2014, https://doi.org/10.5194/acp-14-1717-2014, 2014
D. J. Hoch, J. Buxmann, H. Sihler, D. Pöhler, C. Zetzsch, and U. Platt
Atmos. Meas. Tech., 7, 199–214, https://doi.org/10.5194/amt-7-199-2014, https://doi.org/10.5194/amt-7-199-2014, 2014
R. M. Varma, S. M. Ball, T. Brauers, H.-P. Dorn, U. Heitmann, R. L. Jones, U. Platt, D. Pöhler, A. A. Ruth, A. J. L. Shillings, J. Thieser, A. Wahner, and D. S. Venables
Atmos. Meas. Tech., 6, 3115–3130, https://doi.org/10.5194/amt-6-3115-2013, https://doi.org/10.5194/amt-6-3115-2013, 2013
C. Hörmann, H. Sihler, N. Bobrowski, S. Beirle, M. Penning de Vries, U. Platt, and T. Wagner
Atmos. Chem. Phys., 13, 4749–4781, https://doi.org/10.5194/acp-13-4749-2013, https://doi.org/10.5194/acp-13-4749-2013, 2013
H.-P. Dorn, R. L. Apodaca, S. M. Ball, T. Brauers, S. S. Brown, J. N. Crowley, W. P. Dubé, H. Fuchs, R. Häseler, U. Heitmann, R. L. Jones, A. Kiendler-Scharr, I. Labazan, J. M. Langridge, J. Meinen, T. F. Mentel, U. Platt, D. Pöhler, F. Rohrer, A. A. Ruth, E. Schlosser, G. Schuster, A. J. L. Shillings, W. R. Simpson, J. Thieser, R. Tillmann, R. Varma, D. S. Venables, and A. Wahner
Atmos. Meas. Tech., 6, 1111–1140, https://doi.org/10.5194/amt-6-1111-2013, https://doi.org/10.5194/amt-6-1111-2013, 2013
K. Großmann, U. Frieß, E. Peters, F. Wittrock, J. Lampel, S. Yilmaz, J. Tschritter, R. Sommariva, R. von Glasow, B. Quack, K. Krüger, K. Pfeilsticker, and U. Platt
Atmos. Chem. Phys., 13, 3363–3378, https://doi.org/10.5194/acp-13-3363-2013, https://doi.org/10.5194/acp-13-3363-2013, 2013
P. Lübcke, N. Bobrowski, S. Illing, C. Kern, J. M. Alvarez Nieves, L. Vogel, J. Zielcke, H. Delgado Granados, and U. Platt
Atmos. Meas. Tech., 6, 677–696, https://doi.org/10.5194/amt-6-677-2013, https://doi.org/10.5194/amt-6-677-2013, 2013
Related subject area
Volcanology
Lahar events in the last 2000 years from Vesuvius eruptions – Part 2: Formulation and validation of a computational model based on a shallow layer approach
Lahar events in the last 2000 years from Vesuvius eruptions – Part 3: Hazard assessment over the Campanian Plain
Lahar events in the last 2000 years from Vesuvius eruptions – Part 1: Distribution and impact on densely inhabited territory estimated from field data analysis
Impact of permeability evolution in igneous sills on hydrothermal flow and hydrocarbon transport in volcanic sedimentary basins
Anatomy of a high-silica eruption as observed by a local seismic network: the June 2011 Puyehue–Cordón Caulle event (southern Andes, Chile)
Transient conduit permeability controlled by a shift between compactant shear and dilatant rupture at Unzen volcano (Japan)
Physical and mechanical rock properties of a heterogeneous volcano: the case of Mount Unzen, Japan
Reproducing pyroclastic density current deposits of the 79 CE eruption of the Somma–Vesuvius volcano using the box-model approach
Analysing stress field conditions of the Colima Volcanic Complex (Mexico) by integrating finite-element modelling (FEM) simulations and geological data
Comment on “Estimating the depth and evolution of intrusions at resurgent calderas: Los Humeros (Mexico)” by Urbani et al. (2020)
Cyclic activity of the Fuego de Colima volcano (Mexico): insights from satellite thermal data and nonlinear models
Extrusion dynamics of deepwater volcanoes revealed by 3-D seismic data
A revised map of volcanic units in the Oman ophiolite: insights into the architecture of an oceanic proto-arc volcanic sequence
On the link between Earth tides and volcanic degassing
Failure criteria for porous dome rocks and lavas: a study of Mt. Unzen, Japan
A review of laboratory and numerical modelling in volcanology
Integrating field, textural, and geochemical monitoring to track eruption triggers and dynamics: a case study from Piton de la Fournaise
Periodicity in the BrO∕SO2 molar ratios in the volcanic gas plume of Cotopaxi and its correlation with the Earth tides during the eruption in 2015
Increasing CO2 flux at Pisciarelli, Campi Flegrei, Italy
Dynamics and style transition of a moderate, Vulcanian-driven eruption at Tungurahua (Ecuador) in February 2014: pyroclastic deposits and hazard considerations
Inelastic compaction and permeability evolution in volcanic rock
Eruptive shearing of tube pumice: pure and simple
Numerical models for ground deformation and gravity changes during volcanic unrest: simulating the hydrothermal system dynamics of a restless caldera
Repetitive fracturing during spine extrusion at Unzen volcano, Japan
Poroelastic responses of confined aquifers to subsurface strain and their use for volcano monitoring
Revisiting the statistical analysis of pyroclast density and porosity data
Volcanological aspects of the northwest region of Paraná continental flood basalts (Brazil)
Characterisation of the magmatic signature in gas emissions from Turrialba Volcano, Costa Rica
Morphology and surface features of olivine in kimberlite: implications for ascent processes
Seismogenic frictional melting in the magmatic column
The ring-shaped thermal field of Stefanos crater, Nisyros Island: a conceptual model
New insights on the occurrence of peperites and sedimentary deposits within the silicic volcanic sequences of the Paraná Magmatic Province, Brazil
The permeability and elastic moduli of tuff from Campi Flegrei, Italy: implications for ground deformation modelling
Can vesicle size distributions assess eruption intensity during volcanic activity?
Quantification of magma ascent rate through rockfall monitoring at the growing/collapsing lava dome of Volcán de Colima, Mexico
Bromine monoxide / sulphur dioxide ratios in relation to volcanological observations at Mt. Etna 2006–2009
New developments in the analysis of column-collapse pyroclastic density currents through numerical simulations of multiphase flows
Remobilization of silicic intrusion by mafic magmas during the 2010 Eyjafjallajökull eruption
First observational evidence for the CO2-driven origin of Stromboli's major explosions
Rheological control on the dynamics of explosive activity in the 2000 summit eruption of Mt. Etna
The stochastic quantization method and its application to the numerical simulation of volcanic conduit dynamics under random conditions
Mattia de' Michieli Vitturi, Antonio Costa, Mauro A. Di Vito, Laura Sandri, and Domenico M. Doronzo
Solid Earth, 15, 437–458, https://doi.org/10.5194/se-15-437-2024, https://doi.org/10.5194/se-15-437-2024, 2024
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We present a numerical model for lahars generated by the mobilization of tephra deposits from a reference size eruption at Somma–Vesuvius. The paper presents the model (pyhsics and numerics) and a sensitivity analysis of the processes modelled, numerical schemes, and grid resolution. This work provides the basis for application to hazard quantification for lahars in the Vesuvius area. To this end, we rely on results of the two companion papers (Part 1 on field data, Part 3 on hazard maps).
Laura Sandri, Mattia de' Michieli Vitturi, Antonio Costa, Mauro Antonio Di Vito, Ilaria Rucco, Domenico Maria Doronzo, Marina Bisson, Roberto Gianardi, Sandro de Vita, and Roberto Sulpizio
Solid Earth, 15, 459–476, https://doi.org/10.5194/se-15-459-2024, https://doi.org/10.5194/se-15-459-2024, 2024
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We study the lahar hazard due to the remobilization of tephra deposits from reference eruptions at Somma–Vesuvius. To this end, we rely on the results of two companion papers dealing with field data and model calibration and run hundreds of simulations from the catchments around the target area to capture the uncertainty in the initial parameters. We process the simulations to draw maps of the probability of overcoming thresholds in lahar flow thickness and dynamic pressure relevant for risk.
Mauro Antonio Di Vito, Ilaria Rucco, Sandro de Vita, Domenico Maria Doronzo, Marina Bisson, Mattia de' Michieli Vitturi, Mauro Rosi, Laura Sandri, Giovanni Zanchetta, Elena Zanella, and Antonio Costa
Solid Earth, 15, 405–436, https://doi.org/10.5194/se-15-405-2024, https://doi.org/10.5194/se-15-405-2024, 2024
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We study the distribution of two historical pyroclastic fall–flow and lahar deposits from the sub-Plinian Vesuvius eruptions of 472 CE Pollena and 1631. The motivation comes directly from the widely distributed impact that both the eruptions and lahar phenomena had on the Campanian territory, not only around the volcano but also down the nearby Apennine valleys. Data on about 500 stratigraphic sections and modeling allowed us to evaluate the physical and dynamical impact of these phenomena.
Ole Rabbel, Jörg Hasenclever, Christophe Y. Galerne, Olivier Galland, Karen Mair, and Octavio Palma
Solid Earth, 14, 625–646, https://doi.org/10.5194/se-14-625-2023, https://doi.org/10.5194/se-14-625-2023, 2023
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This work investigates the interaction between magma in the subsurface and the rocks and fluids that surround it. The study investigates how fluids containing hydrocarbons like methane are moving in the rocks surrounding the magma. We show that the generation of fractures in the cooling magma has a significant impact on the flow paths of the fluid and that some of the hydrocabons may be converted to graphite and stored in the fractures within the intrusions.
Daniel Basualto, Andrés Tassara, Jonathan Lazo-Gil, Luis Franco-Marin, Carlos Cardona, Juan San Martín, Fernando Gil-Cruz, Marcela Calabi-Floddy, and Cristian Farías
Solid Earth, 14, 69–87, https://doi.org/10.5194/se-14-69-2023, https://doi.org/10.5194/se-14-69-2023, 2023
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Infrequent eruptions of acidic magma are one of the most dangerous natural phenomena, but almost none of them have been witnessed by modern science. We present the first systematic characterization of seismicity recorded near an erupting acidic volcano (Cordón Caulle 2011). We define different phases of unrest and eruption, which combined with previous findings allows us to discuss the main processes associated with this type of violent eruption, with implications for their volcanic hazard.
Yan Lavallée, Takahiro Miwa, James D. Ashworth, Paul A. Wallace, Jackie E. Kendrick, Rebecca Coats, Anthony Lamur, Adrian Hornby, Kai-Uwe Hess, Takeshi Matsushima, Setsuya Nakada, Hiroshi Shimizu, Bernhard Ruthensteiner, and Hugh Tuffen
Solid Earth, 13, 875–900, https://doi.org/10.5194/se-13-875-2022, https://doi.org/10.5194/se-13-875-2022, 2022
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Volcanic eruptions are controlled by the presence of gas bubbles in magma, which, in excess, can cause explosions. Eruption models lack an understanding of how gas percolates in magma flowing in a conduit. Here we study gas percolation in magma associated with the 1994–1995 eruption at Mt. Unzen, Japan. The results show that the pathways for gas escape depend on the depth and ascent rate of magma. Pathways closed at depth but opened along fractures when magma ascended rapidly near the surface.
Jackie E. Kendrick, Lauren N. Schaefer, Jenny Schauroth, Andrew F. Bell, Oliver D. Lamb, Anthony Lamur, Takahiro Miwa, Rebecca Coats, Yan Lavallée, and Ben M. Kennedy
Solid Earth, 12, 633–664, https://doi.org/10.5194/se-12-633-2021, https://doi.org/10.5194/se-12-633-2021, 2021
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The last lava dome eruption of Mount Unzen (Japan) ended in 1995, but ongoing instability means much of the area remains an exclusion zone. The rocks in the lava dome impact its stability; heterogeneity (contrasting properties) and anisotropy (orientation-specific properties) can channel fluids and localise deformation, enhancing the risk of lava dome collapse. We recommend using measured material properties to interpret geophysical signals and to model volcanic systems.
Alessandro Tadini, Andrea Bevilacqua, Augusto Neri, Raffaello Cioni, Giovanni Biagioli, Mattia de'Michieli Vitturi, and Tomaso Esposti Ongaro
Solid Earth, 12, 119–139, https://doi.org/10.5194/se-12-119-2021, https://doi.org/10.5194/se-12-119-2021, 2021
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In this paper we test a simplified numerical model for pyroclastic density currents or PDCs (mixtures of hot gas, lapilli and ash moving across the landscape under the effect of gravity). The aim is quantifying the differences between real and modelled deposits of some PDCs of the 79 CE eruption of Vesuvius, Italy. This step is important because in the paper it is demonstrated that this simplified model is useful for constraining input parameters for more computationally expensive models.
Silvia Massaro, Roberto Sulpizio, Gianluca Norini, Gianluca Groppelli, Antonio Costa, Lucia Capra, Giacomo Lo Zupone, Michele Porfido, and Andrea Gabrieli
Solid Earth, 11, 2515–2533, https://doi.org/10.5194/se-11-2515-2020, https://doi.org/10.5194/se-11-2515-2020, 2020
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In this work we provide a 2D finite-element modelling of the stress field conditions around the Fuego de Colima volcano (Mexico) in order to test the response of the commercial Linear Static Analysis software to increasingly different geological constraints. Results suggest that an appropriate set of geological and geophysical data improves the mesh generation procedures and the degree of accuracy of numerical outputs, aimed at more reliable physics-based representations of the natural system.
Gianluca Norini and Gianluca Groppelli
Solid Earth, 11, 2549–2556, https://doi.org/10.5194/se-11-2549-2020, https://doi.org/10.5194/se-11-2549-2020, 2020
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We identified several problems in Urbani et al. (2020), showing that their model does not conform to the age and location of faulting, identification and delimitation of uplifted areas and apical depressions, temperature and lithological well log, and stratigraphic and radiometric data. Published data indicate that the pressurization of the Los Humeros volcanic complex (LHVC) magmatic–hydrothermal system driving resurgence faulting occurs at a greater depth.
Silvia Massaro, Antonio Costa, Roberto Sulpizio, Diego Coppola, and Lucia Capra
Solid Earth, 10, 1429–1450, https://doi.org/10.5194/se-10-1429-2019, https://doi.org/10.5194/se-10-1429-2019, 2019
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The Fuego de Colima volcano (Mexico) shows a complex eruptive history, with periods of rapid and slow lava dome growth punctuated by explosive activity. Here we reconstructed the 1998–2018 average discharge rate by means of satellite thermal data and the literature. Using spectral and wavelet analysis, we found a multi-term cyclic behavior that is in good agreement with numerical modeling, accounting for a variable magmatic feeding system composed of a single or double magma chamber system.
Qiliang Sun, Christopher A.-L. Jackson, Craig Magee, Samuel J. Mitchell, and Xinong Xie
Solid Earth, 10, 1269–1282, https://doi.org/10.5194/se-10-1269-2019, https://doi.org/10.5194/se-10-1269-2019, 2019
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3-D seismic reflection data reveal that deepwater volcanoes have rugged basal contacts, which truncate underlying strata, and erupted lava flows that feed lobate lava fans. The lava flows (> 9 km long) account for 50–97 % of the total erupted volume. This indicates that deepwater volcanic edifices may thus form a minor component (~ 3–50 %) of the extrusive system and that accurate estimates of erupted volume require knowledge of the basal surface of genetically related lava flows.
Thomas M. Belgrano, Larryn W. Diamond, Yves Vogt, Andrea R. Biedermann, Samuel A. Gilgen, and Khalid Al-Tobi
Solid Earth, 10, 1181–1217, https://doi.org/10.5194/se-10-1181-2019, https://doi.org/10.5194/se-10-1181-2019, 2019
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We present an updated geological map of the volcanic rocks present in the north-east Oman mountains. These volcanic rocks erupted at the seafloor, probably above a young subduction zone, and have since been tectonically transported into their accessible position. The updated map allows us to examine the spatial relationships between the different volcanic and geological features, including copper, gold, and chrome deposits. The new map will aid further study in Oman and other similar settings.
Florian Dinger, Stefan Bredemeyer, Santiago Arellano, Nicole Bobrowski, Ulrich Platt, and Thomas Wagner
Solid Earth, 10, 725–740, https://doi.org/10.5194/se-10-725-2019, https://doi.org/10.5194/se-10-725-2019, 2019
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Evidence for tidal impacts on volcanism have been gathered by numerous empirical studies. This paper elucidates whether a causal link from the tidal forces to a variation in the volcanic degassing can be traced analytically. We model the response of a simplified magmatic system to the local tidal gravity variations, find that the tide-induced dynamics may significantly alter the bubble coalescence rate, and discuss the consequences for volcanic degassing behaviour.
Rebecca Coats, Jackie E. Kendrick, Paul A. Wallace, Takahiro Miwa, Adrian J. Hornby, James D. Ashworth, Takeshi Matsushima, and Yan Lavallée
Solid Earth, 9, 1299–1328, https://doi.org/10.5194/se-9-1299-2018, https://doi.org/10.5194/se-9-1299-2018, 2018
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Lava domes are mounds of viscous lava and their collapse can cause deadly pyroclastic flows. This paper looks at the example of Mt. Unzen in Japan. Using novel experimental techniques, we discovered that crystals and bubbles in the lava make it behave differently to what was previously thought and that it becomes weaker and more susceptible to collapse as it cools. This calls for a review of current models, allowing for better failure prediction of lava domes in the future.
Janine L. Kavanagh, Samantha L. Engwell, and Simon A. Martin
Solid Earth, 9, 531–571, https://doi.org/10.5194/se-9-531-2018, https://doi.org/10.5194/se-9-531-2018, 2018
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Modelling has been used in the study of volcanic systems for more than 100 years, building upon the approach first described by Sir James Hall in 1815. Models are informed by observations of volcanic processes in nature, including eye-witness accounts of eruptions, monitoring of active volcanoes, and analysis of ancient deposits. To push the frontiers in volcanology we must adopt a multidisciplinary approach, with more interaction between analogue and numerical modelling communities.
Lucia Gurioli, Andrea Di Muro, Ivan Vlastélic, Séverine Moune, Simon Thivet, Marina Valer, Nicolas Villeneuve, Guillaume Boudoire, Aline Peltier, Patrick Bachèlery, Valérie Ferrazzini, Nicole Métrich, Mhammed Benbakkar, Nicolas Cluzel, Christophe Constantin, Jean-Luc Devidal, Claire Fonquernie, and Jean-Marc Hénot
Solid Earth, 9, 431–455, https://doi.org/10.5194/se-9-431-2018, https://doi.org/10.5194/se-9-431-2018, 2018
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We prove here that macroscopic and microscopic studies of emitted pyroclastic and effusive products provide valuable information to track and understand small explosive eruptions for hazard and risk assessment. This is especially true for Piton de La Fournaise, La Réunion, whose activity has recently been characterized by effusive and mild explosive activity in highly visited areas. We confirm that petrological monitoring is essential to forecast changes in the magmatic system.
Florian Dinger, Nicole Bobrowski, Simon Warnach, Stefan Bredemeyer, Silvana Hidalgo, Santiago Arellano, Bo Galle, Ulrich Platt, and Thomas Wagner
Solid Earth, 9, 247–266, https://doi.org/10.5194/se-9-247-2018, https://doi.org/10.5194/se-9-247-2018, 2018
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We monitored the bromine monoxide-to-sulfur dioxide molar ratio in the effusive gas plume of Cotopaxi volcano in order to gain insight into the geological processes which control the pressure regime of the volcanic system. We observed a conspicuous periodic pattern with a periodicity of about 2 weeks, which significantly correlates with the Earth tidal forcing. Our results support a possible Earth tidal impact on volcanic activity, in particular for the Cotopaxi eruption 2015.
Manuel Queißer, Domenico Granieri, Mike Burton, Fabio Arzilli, Rosario Avino, and Antonio Carandente
Solid Earth, 8, 1017–1024, https://doi.org/10.5194/se-8-1017-2017, https://doi.org/10.5194/se-8-1017-2017, 2017
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Campi Flegrei is a volcanic caldera that is currently in a state of increased unrest. We used a novel remote-sensing approach to measure CO2 fluxes at the Campi Flegrei. Thanks to its comprehensive spatial coverage, the instrument used gives more representative measurements from large regions containing different CO2 sources. We find an increase in CO2 degassing strength. This suggests a greater contribution of the magmatic source to the degassing.
Jorge Eduardo Romero, Guilhem Amin Douillet, Silvia Vallejo Vargas, Jorge Bustillos, Liliana Troncoso, Juan Díaz Alvarado, and Patricio Ramón
Solid Earth, 8, 697–719, https://doi.org/10.5194/se-8-697-2017, https://doi.org/10.5194/se-8-697-2017, 2017
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The 1 February 2014 eruption of the Tungurahua volcano (Ecuador) was the second largest one since the re-awakening in 1999. The eruption showed precursory signs only 48 h before the eruption. The main explosions produced a 13 km eruptive column and pyroclastic density currents that reached the base of the volcano.
Here we document the deposits related to the eruption and infer eruption mechanisms and transport processes.
Jamie I. Farquharson, Patrick Baud, and Michael J. Heap
Solid Earth, 8, 561–581, https://doi.org/10.5194/se-8-561-2017, https://doi.org/10.5194/se-8-561-2017, 2017
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In volcanic rock, permeability is the property that tells us how efficiently fluids such as gas or water can travel through cracks and frozen bubbles in the rock (its porosity) and is important in the context of volcanic activity. This study addresses how permeability evolves under a range of mechanical experimental conditions. We show that with a small amount of porosity loss (compaction), permeability can increase. However, with more compaction, permeability can decrease significantly.
Donald B. Dingwell, Yan Lavallée, Kai-Uwe Hess, Asher Flaws, Joan Marti, Alexander R. L. Nichols, H. Albert Gilg, and Burkhard Schillinger
Solid Earth, 7, 1383–1393, https://doi.org/10.5194/se-7-1383-2016, https://doi.org/10.5194/se-7-1383-2016, 2016
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Here, we use tomography to reconstructed the pores of erupted pumice and understand the evolution of gas bubbles in magma. Analysis of the pore geometry is used to describe whether the pores where aligned by stretching as ascending magma is pulled apart (pure shear) or sheared like a deck of card (simple shear). We conclude that the latter, simple shear, dominates during magma ascent up to the points where magma fragments to cause an explosion.
A. Coco, J. Gottsmann, F. Whitaker, A. Rust, G. Currenti, A. Jasim, and S. Bunney
Solid Earth, 7, 557–577, https://doi.org/10.5194/se-7-557-2016, https://doi.org/10.5194/se-7-557-2016, 2016
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We present a numerical model to evaluate ground deformation and gravity changes as a response of the hydrothermal system perturbation (unrest) in a volcanic area. Temporal evolution of the ground deformation indicates that the contribution of thermal effects to the total uplift is almost negligible with respect to the pore pressure contribution during the first years, of the unrest, but increases in time and becomes dominant after a long period of the simulation.
O. D. Lamb, S. De Angelis, K. Umakoshi, A. J. Hornby, J. E. Kendrick, and Y. Lavallée
Solid Earth, 6, 1277–1293, https://doi.org/10.5194/se-6-1277-2015, https://doi.org/10.5194/se-6-1277-2015, 2015
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In this paper we analyse the seismic record during the extrusion of a lava spine at Unzen volcano, Japan, in 1994. We find two strong groups of similar volcanic earthquakes which, combined with previously published field and experimental observations, we interpret as repetitive fracturing along the margin of the lava spine. This work demonstrates the potential of combining these different approaches for achieving a greater understanding of shallow volcanic processes.
K. Strehlow, J. H. Gottsmann, and A. C. Rust
Solid Earth, 6, 1207–1229, https://doi.org/10.5194/se-6-1207-2015, https://doi.org/10.5194/se-6-1207-2015, 2015
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When magma chambers inflate, they deform the surrounding Earth’s crust. This deformation affects the pore space available for the water in local aquifers, which in turn leads to pressure variations and water table changes. We can observe these changes in wells, and this study investigates if and how we can utilize them for volcano monitoring. Results show that the hydrological response to deformation helps unravelling subsurface magmatic processes, valuable information for eruption forecasting.
B. Bernard, U. Kueppers, and H. Ortiz
Solid Earth, 6, 869–879, https://doi.org/10.5194/se-6-869-2015, https://doi.org/10.5194/se-6-869-2015, 2015
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This paper presents a new methodology to treat statistically pyroclast density and porosity data sets introducing a weighting parameter. It also proposes a stability analysis to check if the sample set is large enough for statistical reliability. Finally we introduce graphical statistics to improve distinction between pyroclastic deposits and understanding of eruptive dynamics. An open source R code is supplied that includes all these features in order to facilitate data processing.
F. Braz Machado, E. Reis Viana Rocha-Júnior, L. Soares Marques, and A. J. Ranalli Nardy
Solid Earth, 6, 227–241, https://doi.org/10.5194/se-6-227-2015, https://doi.org/10.5194/se-6-227-2015, 2015
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This study describes for the first time morphological aspects of lava flows and structural characteristics caused by lava-sediment interaction in the northwestern Paraná continental flood basalts in the southeast of the South American Plate (Brazil). Early Cretaceous (134 to 132Ma) tholeiitic rocks were emplaced on a large intracratonic Paleozoic sedimentary basin (Paraná Basin), mainly covering dry eolian sandstones (Botucatu Formation).
Y. Moussallam, N. Peters, C. Ramírez, C. Oppenheimer, A. Aiuppa, and G. Giudice
Solid Earth, 5, 1341–1350, https://doi.org/10.5194/se-5-1341-2014, https://doi.org/10.5194/se-5-1341-2014, 2014
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In this paper we characterise the flux and composition of the gas emissions from Turrialba Volcano. We show that the measured gas signature provides evidence that Turrialba Volcano has entered an open-vent configuration with magmatic gases being emitted. This suggests that the hydrothermal system at the summit is quickly drying up and that the system is moving from a hydrothermal to a magmatic end member with implications for short-term monitoring and possible evolution of the state of unrest.
T. J. Jones, J. K. Russell, L. A. Porritt, and R. J. Brown
Solid Earth, 5, 313–326, https://doi.org/10.5194/se-5-313-2014, https://doi.org/10.5194/se-5-313-2014, 2014
J. E. Kendrick, Y. Lavallée, K.-U. Hess, S. De Angelis, A. Ferk, H. E. Gaunt, P. G. Meredith, D. B. Dingwell, and R. Leonhardt
Solid Earth, 5, 199–208, https://doi.org/10.5194/se-5-199-2014, https://doi.org/10.5194/se-5-199-2014, 2014
M. Pantaleo and T. R. Walter
Solid Earth, 5, 183–198, https://doi.org/10.5194/se-5-183-2014, https://doi.org/10.5194/se-5-183-2014, 2014
A. C. F. Luchetti, A. J. R. Nardy, F. B. Machado, J. E. O. Madeira, and J. M. Arnosio
Solid Earth, 5, 121–130, https://doi.org/10.5194/se-5-121-2014, https://doi.org/10.5194/se-5-121-2014, 2014
M. J. Heap, P. Baud, P. G. Meredith, S. Vinciguerra, and T. Reuschlé
Solid Earth, 5, 25–44, https://doi.org/10.5194/se-5-25-2014, https://doi.org/10.5194/se-5-25-2014, 2014
A. LaRue, D. R. Baker, M. Polacci, P. Allard, and N. Sodini
Solid Earth, 4, 373–380, https://doi.org/10.5194/se-4-373-2013, https://doi.org/10.5194/se-4-373-2013, 2013
S. B. Mueller, N. R. Varley, U. Kueppers, P. Lesage, G. Á. Reyes Davila, and D. B. Dingwell
Solid Earth, 4, 201–213, https://doi.org/10.5194/se-4-201-2013, https://doi.org/10.5194/se-4-201-2013, 2013
N. Bobrowski and G. Giuffrida
Solid Earth, 3, 433–445, https://doi.org/10.5194/se-3-433-2012, https://doi.org/10.5194/se-3-433-2012, 2012
S. Lepore and C. Scarpati
Solid Earth, 3, 161–173, https://doi.org/10.5194/se-3-161-2012, https://doi.org/10.5194/se-3-161-2012, 2012
O. Sigmarsson, I. Vlastelic, R. Andreasen, I. Bindeman, J.-L. Devidal, S. Moune, J. K. Keiding, G. Larsen, A. Höskuldsson, and Th. Thordarson
Solid Earth, 2, 271–281, https://doi.org/10.5194/se-2-271-2011, https://doi.org/10.5194/se-2-271-2011, 2011
A. Aiuppa, M. Burton, P. Allard, T. Caltabiano, G. Giudice, S. Gurrieri, M. Liuzzo, and G. Salerno
Solid Earth, 2, 135–142, https://doi.org/10.5194/se-2-135-2011, https://doi.org/10.5194/se-2-135-2011, 2011
D. Giordano, M. Polacci, P. Papale, and L. Caricchi
Solid Earth, 1, 61–69, https://doi.org/10.5194/se-1-61-2010, https://doi.org/10.5194/se-1-61-2010, 2010
E. Peruzzo, M. Barsanti, F. Flandoli, and P. Papale
Solid Earth, 1, 49–59, https://doi.org/10.5194/se-1-49-2010, https://doi.org/10.5194/se-1-49-2010, 2010
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